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BestCrosswords.com - "Hoodoo Magic" by Frank Virzi on 4/2/2017 [moderate]
Across 1- Neeson of "Schindler's List"; 5- Perfect for picking; 9- Biotite and phlogopite; 14- Site of Cyclops' smithy; 15- Off-the-wall response?; 16- Praying figure, in art; 17- *Question to a caller asking someone about her running refrigerator or Prince Albert in a can; 19- Actress Lisi; 20- In need of some hammering out; 21- The maximum one for a goldfish is 25 years; 23- Ship's departure?; 24- *"___ Congress": Harry Truman's nickname for lawmakers during the 1948 election; 25- Advanced study group; 28- Author Asquith of children's books; 29- Cargo on the Spanish Main; 30- Cook up, so to speak; 33- Hungarian city near Miskolc; 37- *"That's supposed to scare me?"; 40- Part of NBA: Abbr.; 41- Removed by a coup; 42- Soul, to Sartre; 43- "Zero K" author DeLillo; 45- Weeks in Madrid; 47- *1970 tearjerker set at Harvard; 52- Western capital: Abbr.; 53- Vanquish; 54- Company formed by the 1986 Sperry-Burroughs merger; 57- Buoyant wood sometimes used in rafts; 58- Legendary bluesman who wrote the classic song with the title formed by the starts of the starred answers; 60- Knight's "suit"; 61- Herb Alpert's #1 jazz-funk hit of 1979; 62- Diner sign; 63- "___ Hope": '70s-'80s soap; 64- Angled annexes; 65- Inspired with love, old-style;   Down 1- Bawdy; 2- Spillane's "____ Jury"; 3- "Primary Colors" author, as originally published in 1996; 4- Drink sometimes served in a pineapple; 5- On Soc. Sec., perhaps; 6- First person in Germany?; 7- American inventor and television pioneer Farnsworth; 8- Red dye used in a biology lab; 9- Take up new residence in; 10- It surrounds the Isle of Man; 11- Eight small bones that connect the hand to the forearm; 12- 2001 Nobel Peace Prize winner Kofi; 13- Ford muscle car, to devotees; 18- Like many monograms on clothing; 22- Divine; 24- Sch. in Madison, NJ; 25- Tofu source; 26- Arrow-shooting Greek god; 27- Enlarge, as a home; 31- Sighs of relief; 32- Hotsy-___; 34- One of Lou Gehrig's 23 big blasts in his career; 35- Title character from the village of Highbury, 1815; 36- Some distillery products; 38- "Nothing Left Unsaid: Gloria Vanderbilt & ___ Cooper": 2016 HBO documentary; 39- Onetime Secretary of State Muskie; 44- "La La Land" sextet; 46- Opening monologues of "Ferris Bueller's Day Off" and "House of Cards"; 47- Kind of pneumonia; 48- One end of a fallopian tube; 49- Roxie's dance partner in "Chicago"; 50- Card game of Spanish origin played with a 40-card deck; 51- Work on, as a creaky hinge; 54- 180-degree turns, in slang; 55- Himalayan legend; 56- Part of iOS; 59- Certain Internet connection: Abbr.;