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BestCrosswords.com - "Head Scratchers" by Frank Virzi on 11/1/2014 [moderate]
Across 1- City that's about 43 miles west of Florence; 5- Final authority; 10- "Washington Week" airer; 13- PFCs' addresses; 14- Advance again; 15- "The Fall of the House of Usher" monogram; 16- Song with the line, "Hey I just met you, and this is crazy"; 18- Start to dominate?; 19- Ta-tas in Toulouse; 20- '60s-'70s Italian prime minister Aldo; 21- Ham, to Noah; 22- Toon frame; 23- All females, as a group; 25- Like some baseball teams; 28- On the briny; 29- Granola grain; 30- Mahler's "Das Lied von der ____"; 32- Not very many; 36- Cinnabar, e.g.; 37- Feature of some classic cars; 41- Dockworkers' org.; 42- "Charlie's Angels" actress; 44- "Encore!"; 45- Cath. or Luth.; 46- Car-racing org.; 50- Prepares to go?; 52- "Notre Dame Victory March" or "Hail Purdue," e.g.; 56- Tiny tyke; 57- Dawg; 58- Pins and needles holder; 59- Deli machine; 62- 20-vol. work; 63- Practice what one preaches; 65- L-P filler; 66- Make precious; 67- Langston Hughes poem; 68- Take a chance; 69- Symbol of freshness; 70- Form 1040 IDs;   Down 1- Square-headed rodent; 2- April 2010 Apple release; 3- Sought earnestly; 4- Out; 5- Place for a father-to-be: Abbr.; 6- 1836 battle site; 7- Player of a 1733 Montagnana cello named Petunia; 8- Native Israelis; 9- Final score of the second MLB All-Star Game played at Fenway Park in 1961; 10- "More bounce to the ounce" sloganeer, once; 11- Red or robber follower; 12- Forgo frugality; 14- Hi-___ graphics; 17- "Business in the front, party in the back" hair style; 23- Gully that's usually dry; 24- "The Jungle Book" creature voiced by Sterling Holloway; 25- Word with bar or box; 26- Avis lead-in; 27- Stat for Jon Lester; 31- "I will fasten on this sleeve of thine: thou art an ___, my husband, I a vine": Shakespeare; 33- Coolidge's Tiger and Clinton's Socks - and a hint to the theme of this puzzle; 34- Completion of Robt.'s signature; 35- Poet Whitman; 38- Verne traveler; 39- Choler; 40- Get under the skin of; 43- "I am such a dope!"; 47- Stinko; 48- Capital of Kazakhstan; 49- "Will you let me?"; 51- "You're right after all"; 52- Euphemism for a word seldom heard in PG-13 movies; 53- Goodnight girl; 54- Beckett's no-show; 55- Some sneaks; 59- NYSE unit; 60- Carolina university; 61- Bygone theaters; 64- Scotland's longest river;