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BestCrosswords.com - "Themeless 37" by Patricia Wells on 1/14/2014 [moderate]
Across 1- End ____; 5- Type of insulation; 9- Dry roast; 14- Performance-enhancing drugs; 15- Psychic sight; 16- It's a lizard; 17- It's overhead; 18- Military rank symbol; 19- One of the powers that be, in India; 20- Pay dirt; 21- What you did before Christmas ? (part 1); 23- A weather center; 24- French composer Erik; 26- Milli Vanilli's Morvan; 28- High-ranking post in the DOJ; 30- High pressured stream of liquid; 32- Adjutant; 36- Egyptian Christian; 39- Requirement; 41- Leader in his field, perhaps; 42- Moonfish; 43- Part 2 of 21 across; 45- Extend credit; 46- Ancient scientists; 47- Former Brown's quarterback, Graham; 48- Tributes; 49- Nautical direction; 50- A kind of ash; 51- Part 3 of 21 across; 53- Aviation branch of the USDOT; 55- They reverse previous instructions; 59- Defraud; 62- Part 4 of 21 across; 67- Vital force of Chinese medicine; 68- Employ again; 70- Conductor cable; 71- Unit of pressure; 72- The anchor is barely aweigh; 73- Physician-scientists honor society, init.; 74- Medicinal plant; 75- The right to take or leave (part 1); 76- A network of tunnels; 77- Part 2 of 75 across;   Down 1- They add value; 2- Italian theater; 3- Risky trapeze setup (2wds); 4- Suffix meaning "the most"; 5- Diss; 6- Camera setting; 7- Big fat mouth; 8- Emergency shelter; 9- Giant bamboo eater; 10- Literary olio; 11- Morning coat; 12- Sate overly; 13- Small garden shrub; 21- China e.g.; 22- Online payment, init.; 25- Name stealer; 27- Washington fiasco; 29- Wildebeest; 30- Breakwater; 31- Modify; 33- Kind of tea; 34- Ready to eat; 35- Bacon pieces; 36- Medically induced sleep e.g.; 37- Sandstone gem; 38- Call for; 40- Form of ether; 44- Irish post hole spade; 50- Wide's partner; 52- Exterior sound system component, init; 54- Highly skilled; 56- Bacteria discovered by Theodor Escherich; 57- Pulsate; 58- Fathers; 59- Tennis's Steffi; 60- Creature of legend; 61- Sound of contentment; 63- Wood sorrels; 64- Sit; 65- Treaty; 66- A way out; 69- Family nickname; 71- Smidgen;