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BestCrosswords.com - "Rhyming Guys (11005)" by Gareth Bain on 2/14/2011 [moderate]
Across 1- Hurtled; 5- "The Highwayman," for one; 9- Puts in stitches; 13- Register with the ear; 14- Tete concoctions; 16- PBS shower in NYC; 17- Gillette brand; 18- The "Hostess with the Mostest"; 20- Cry given with a leash in hand [Hi BFM!]; 22- "Anna and the King" actress; 23- Puzzle; 25- Plentiful marine flora; 26- ___-ray Disc; 28- Decoration for a general; 31- Radio network with pledge drives; 32- Celebrated; 34- Chill out; 36- Upset the composure of; 37- Western accent; 39- Flows back; 43- Weak at the ___; 45- Thin porridge; 46- ___ Kippur; 49- Policeman; 52- Detective ___ Curtis (Benjamin Bratt role); 53- Some sneakers; 55- Rabbit ears; 57- Time of crisis?; 60- Modern fashion statement; 63- Author of Sunday crosswords who voiced himself on The Simpsons; 65- It cooks your goose; 66- Singer Brickell who married Paul Simon; 67- Sag; 68- City on the Salt River; 69- Emulates Robin Hood; 70- Co-owner of the Hubble Space Telescope; 71- Aide (abbr.);   Down 1- The S of GBS; 2- Fur doesn't fly with this org.; 3- Disgraced Agriculture secretary during the Nixon administration [BTW, yes, I needed to look him up to complete this theme]; 4- Piratical Sir Francis; 5- Find your voice; 6- Russian vacation city; 7- Poetic contraction; 8- "Scary Spice"; 9- Imitate a cell in a hypotonic environment; 10- Rank below Lieutenant Junior Grade in the USN; 11- Messy diner's accessory; 12- Old hand; 15- Ray's home; 19- Mazda MX-5; 21- Sent a message via Googletalk; 24- Location of the Alps and the Himalayas; 26- Supertight pal; 27- Idyll location; 29- Wallace who wrote Ben-Hur; 30- Shape formed by a right angle; 33- "A mouse!" in comics; 35- Gen-___; 37- ___ Leppard; 38- One who may call for icing; 40- Folk singer who won an Oscar in 1958; 41- Spellers' face-off; 42- Sylvester's nickname; 44- Formal refusal; 45- "Get a ___!"; 46- Kvetch; 47- City in north-west Spain; 48- Leaf's divider; 50- Unwieldy strings; 51- Rust Belt city; 54- The Dead Kennedys' "California Uber ___"; 56- Bacon-frying byproduct; 58- 61D, notably; 59- Make bread; 61- "Untouchable" one; 62- Biting pest; 64- Indian state that once belonged to Portugal;